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Temperature dependent luminescence and dephasing of gold nanorods

  • In this study we demonstrate the impact of temperature on the luminescence emission of plasmonic nanoparticles. We examine the optical properties of single gold nanorods (GNRs) in the temperature range 1.6–295 K by confocal microscopy. Decreasing temperature leads to a reduction of the full width at half-maximum (fwhm) of the luminescence spectra, thus we can conclude that the damping of the plasmonic oscillation is strongly reduced. The main contribution to the dephasing mechanism is electron–phonon scattering and we are able to determine its contribution to the dephasing using quantitative simulations, which can describe the temperature dependent dephasing of plasmonic nanoparticles.

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Metadaten
Author of HS ReutlingenWackenhut, Frank
DOI:https://doi.org/10.1021/jp407178u
ISSN:1932-7455
Published in:The journal of physical chemistry C
Publisher:American Chemical Society
Place of publication:Washington, DC
Document Type:Journal article
Language:English
Publication year:2013
Volume:117
Issue:41
Page Number:7
First Page:21476
Last Page:21482
DDC classes:530 Physik
540 Chemie
Open access?:Nein
Licence (German):License Logo  In Copyright - Urheberrechtlich geschützt